Qureshi, N., Drees, Y., Werner, J., Wurmehl, S., Hess, C., Klingeler, R., Buechner, B., Fernandez-Diaz, M. T. and Braden, M. (2010). Crystal and magnetic structure of the oxypnictide superconductor LaFeAsO1-xFx: A neutron-diffraction study. Phys. Rev. B, 82 (18). COLLEGE PK: AMER PHYSICAL SOC. ISSN 2469-9969

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Abstract

High-resolution and high-flux neutron as well as x-ray powder-diffraction experiments were performed on the oxypnictide series LaO1-xFxFeAs with 0 <= x <= 0.15 in order to study the crystal and magnetic structure. The magnetic symmetry of the undoped compound corresponds to those reported for REOFeAs (with RE a rare earth) and for AFe(2)As(2)(A=Ba, Sr) materials. We find an ordered magnetic moment of 0.63(1) mu B at 2 K in LaOFeAs, which is significantly larger than the values previously reported for this compound. A sizable ordered magnetic moment is observed up to a F doping of 4.5% whereas there is no magnetic order for a sample with a F concentration of x=0.06. In the undoped sample, several interatomic distances and FeAs4 tetrahedra angles exhibit pronounced anomalies connected with the broad structural transition and with the onset of magnetism supporting the idea of strong magnetoelastic coupling in this material.

Item Type: Journal Article
Creators:
CreatorsEmailORCIDORCID Put Code
Qureshi, N.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Drees, Y.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Werner, J.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Wurmehl, S.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Hess, C.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Klingeler, R.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Buechner, B.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Fernandez-Diaz, M. T.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Braden, M.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
URN: urn:nbn:de:hbz:38-492542
DOI: 10.1103/PhysRevB.82.184521
Journal or Publication Title: Phys. Rev. B
Volume: 82
Number: 18
Date: 2010
Publisher: AMER PHYSICAL SOC
Place of Publication: COLLEGE PK
ISSN: 2469-9969
Language: English
Faculty: Unspecified
Divisions: Unspecified
Subjects: no entry
Uncontrolled Keywords:
KeywordsLanguage
ELECTRONIC PHASE-DIAGRAM; IRONMultiple languages
Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed MatterMultiple languages
URI: http://kups.ub.uni-koeln.de/id/eprint/49254

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