Universität zu Köln

Jager, Christina, Bruneau, Cloe, Wagner, Philip K., Prechtl, Martin H. G. ORCID: 0000-0003-2155-8006 and Deska, Jan (2021). Methanol-Driven Oxidative Rearrangement of Biogenic Furans - Enzyme Cascades vs. Photobiocatalysis. Front. Chem., 9. LAUSANNE: FRONTIERS MEDIA SA. ISSN 2296-2646

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Abstract

The oxidative ring expansion of bio-derived furfuryl alcohols to densely functionalized six-membered O-heterocycles represents an attractive strategy in the growing network of valorization routes to synthetic building blocks out of the lignocellulosic biorefinery feed. In this study, two scenarios for the biocatalytic Achmatowicz-type rearrangement using methanol as terminal sacrificial reagent have been evaluated, comparing multienzymatic cascade designs with a photo-bio-coupled activation pathway.

Item Type:	Journal Article
Creators:	Creators Email ORCID ORCID Put Code Jager, Christina UNSPECIFIED UNSPECIFIED UNSPECIFIED Bruneau, Cloe UNSPECIFIED UNSPECIFIED UNSPECIFIED Wagner, Philip K. UNSPECIFIED UNSPECIFIED UNSPECIFIED Prechtl, Martin H. G. UNSPECIFIED orcid.org/0000-0003-2155-8006 UNSPECIFIED Deska, Jan UNSPECIFIED UNSPECIFIED UNSPECIFIED
URN:	urn:nbn:de:hbz:38-582598
DOI:	10.3389/fchem.2021.635883
Journal or Publication Title:	Front. Chem.
Volume:	9
Date:	2021
Publisher:	FRONTIERS MEDIA SA
Place of Publication:	LAUSANNE
ISSN:	2296-2646
Language:	English
Faculty:	Unspecified
Divisions:	Unspecified
Subjects:	no entry
Uncontrolled Keywords:	Keywords Language Chemistry, Multidisciplinary Multiple languages
URI:	http://kups.ub.uni-koeln.de/id/eprint/58259