Sterzi, A., Manzoni, G., Sbuelz, L., Cilento, F., Zacchigna, M., Bugnon, Ph, Magrez, A., Berger, H., Crepaldi, A. and Parmigiani, F. (2017). Bulk diffusive relaxation mechanisms in optically excited topological insulators. Phys. Rev. B, 95 (11). COLLEGE PK: AMER PHYSICAL SOC. ISSN 2469-9969

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Abstract

The possibility to inject spin currents in topological insulators (TIs) by ultrashort optical pulses has stimulated intense studies of their out-of-equilibrium electronic properties. However, a comprehensive description of the electronic relaxation dynamics has been elusive, so far. In order to reveal the role of the bulk and surface states in the microscopic scattering mechanisms, we have investigated, by means of time-and angle-resolved photoemission spectroscopy, a wide set of TIs. These have been selected in order to display different positions of the Fermi energy (E-F) within the bulk band structure. When three-dimensional bulk states lie at E-F, we observe a fast relaxation dynamics with a characteristic time scale of a few picoseconds (ps). On the contrary, a long lasting excited state is recorded when only the two-dimensional surface state crosses E-F. These findings suggest the important role played by spatial diffusion in the direction orthogonal to the surface in governing the relaxation mechanisms. We propose that this electron diffusive mechanism is driven by the optically induced temperature gradient that is at play only for electrons residing in bulk states.

Item Type: Journal Article
Creators:
CreatorsEmailORCIDORCID Put Code
Sterzi, A.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Manzoni, G.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Sbuelz, L.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Cilento, F.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Zacchigna, M.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Bugnon, PhUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Magrez, A.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Berger, H.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Crepaldi, A.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Parmigiani, F.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
URN: urn:nbn:de:hbz:38-236285
DOI: 10.1103/PhysRevB.95.115431
Journal or Publication Title: Phys. Rev. B
Volume: 95
Number: 11
Date: 2017
Publisher: AMER PHYSICAL SOC
Place of Publication: COLLEGE PK
ISSN: 2469-9969
Language: English
Faculty: Unspecified
Divisions: Unspecified
Subjects: no entry
Uncontrolled Keywords:
KeywordsLanguage
ELECTRON THERMALIZATION; SURFACE; DYNAMICS; ARPESMultiple languages
Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed MatterMultiple languages
Refereed: Yes
URI: http://kups.ub.uni-koeln.de/id/eprint/23628

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