Sharma, Shivani, Adroja, D. T., Ritter, C., Khalyavin, D., Manuel, P., Stenning, Gavin B. G., Sundaresan, A., Hillier, A. D., Deen, P. P., Khomskii, D., I and Langridge, S. (2020). Magnetic ground state of the ordered double-perovskite Sr2YbRuO6: Two magnetic transitions. Phys. Rev. B, 102 (13). COLLEGE PK: AMER PHYSICAL SOC. ISSN 2469-9969
Full text not available from this repository.Abstract
Comprehensive muon-spin-rotation/relaxation (mu SR) and neutron powder-diffraction (NPD) studies supported via bulk measurements have been performed on the ordered double-perovskite Sr2YbRuO6 to investigate the nature of the magnetic ground state. Two sharp transitions at T-N1 similar to 42 K and T-N2 similar to 36 K have been observed in the static and dynamic magnetization measurements, coinciding with the heat-capacity data. In order to confirm the origin of the observed phase transitions and the magnetic ground state, microscopic evidences are presented here. An initial indication of long-range magnetic ordering comes from a sharp drop in the muon initial asymmetry and a peak in the relaxation rate near T-N1. NPD confirms that the magnetic ground state of Sr2YbRuO6 consists of an antiferromagnetic (AFM) structure with interpenetrating lattices of parallel Yb3+ and Ru5+ moments lying in the ab plane and adopting an A-type AFM structure. Intriguingly, a small but remarkable change is observed in the long-range ordering parameters at T-N2 confirming the presence of a weak spin reorientation (i.e., change in spin configuration) transition of Ru and Yb moments, as well as a change in the magnetic moment evolution of the Yb3+ spins at T-N2. The temperature-dependent behavior of the Yb3+ and Ru5+ moments suggests that the 4d electrons of Ru5+ play a dominating role in stabilizing the long-range-ordered magnetic ground state in the double-perovskite Sr2YbRuO6 whereas only the Yb3+ moments show an arrest at T-N2. The observed magnetic structure and the presence of a ferromagnetic interaction between Ru and Yb ions are explained with use of the Goodenough-Kanamori-Anderson rules. Possible reasons for the presence of the second magnetic phase transition and of a compensation point in the magnetization data are linked to competing mechanisms of magnetic anisotropy.
| Item Type: | Journal Article | ||||||||||||||||||||||||||||||||||||||||||||||||
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| URN: | urn:nbn:de:hbz:38-315381 | ||||||||||||||||||||||||||||||||||||||||||||||||
| DOI: | 10.1103/PhysRevB.102.134412 | ||||||||||||||||||||||||||||||||||||||||||||||||
| Journal or Publication Title: | Phys. Rev. B | ||||||||||||||||||||||||||||||||||||||||||||||||
| Volume: | 102 | ||||||||||||||||||||||||||||||||||||||||||||||||
| Number: | 13 | ||||||||||||||||||||||||||||||||||||||||||||||||
| Date: | 2020 | ||||||||||||||||||||||||||||||||||||||||||||||||
| Publisher: | AMER PHYSICAL SOC | ||||||||||||||||||||||||||||||||||||||||||||||||
| Place of Publication: | COLLEGE PK | ||||||||||||||||||||||||||||||||||||||||||||||||
| ISSN: | 2469-9969 | ||||||||||||||||||||||||||||||||||||||||||||||||
| Language: | English | ||||||||||||||||||||||||||||||||||||||||||||||||
| Faculty: | Unspecified | ||||||||||||||||||||||||||||||||||||||||||||||||
| Divisions: | Unspecified | ||||||||||||||||||||||||||||||||||||||||||||||||
| Subjects: | no entry | ||||||||||||||||||||||||||||||||||||||||||||||||
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| URI: | http://kups.ub.uni-koeln.de/id/eprint/31538 |
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