Universität zu Köln

Hell, Martin G., Falke, Yannic, Bliesener, Andrea, Ehlen, Niels, Senkovskiy, Boris V. ORCID: 0000-0003-1443-6780, Szkopek, Thomas and Grueneis, Alexander (2018). Combined Ultra High Vacuum Raman and Electronic Transport Characterization of Large-Area Graphene on SiO2. Phys. Status Solidi B-Basic Solid State Phys., 255 (12). WEINHEIM: WILEY-V C H VERLAG GMBH. ISSN 1521-3951

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Abstract

An original experimental setup which allows for simultaneous sample characterization by Raman spectroscopy and electronic tranport in ultra-high vacuum at low temperatures is presented. We show the applicability of this setup for the case of graphene that is transferred from an Ir(111) single crystal onto SiO2. The transfer of graphene is carried out using a water-promoted electrochemical bubbling technique which is applied to graphene/Ir for the first time. The characterization prior to the transfer includes electron diffraction, photoemission spectroscopy and Raman spectroscopy using ultraviolet excitation. Following the transfer procedure, the graphene layer is electrically contacted and mounted onto a special sample carrier. This carrier allows for combined Raman and transport measurements inside an ultra high vacuum (UHV) system. UHV Raman mapping reveals a large area homogeneous graphene quality over several mm(2) characterized by a D/G intensity ratio less than 0.1. UHV electrical characterization of transferred graphene in a field effect transistor geometry yields a carrier mobility of 675 cm(2) V-1 s(-1). Upon alkali metal doping in UHV conditions using a Cs getter, a decrease of the 4-point resistance from above 2500 omega to below 10 omega is observed. The presented approach paves the way for future combined UHV Raman and transport characterization of two-dimensional materials that are doped into superconducting or charge-density-wave ground states.

Item Type:	Journal Article
Creators:	Creators Email ORCID ORCID Put Code Hell, Martin G. UNSPECIFIED UNSPECIFIED UNSPECIFIED Falke, Yannic UNSPECIFIED UNSPECIFIED UNSPECIFIED Bliesener, Andrea UNSPECIFIED UNSPECIFIED UNSPECIFIED Ehlen, Niels UNSPECIFIED UNSPECIFIED UNSPECIFIED Senkovskiy, Boris V. UNSPECIFIED orcid.org/0000-0003-1443-6780 UNSPECIFIED Szkopek, Thomas UNSPECIFIED UNSPECIFIED UNSPECIFIED Grueneis, Alexander UNSPECIFIED UNSPECIFIED UNSPECIFIED
URN:	urn:nbn:de:hbz:38-163336
DOI:	10.1002/pssb.201800456
Journal or Publication Title:	Phys. Status Solidi B-Basic Solid State Phys.
Volume:	255
Number:	12
Date:	2018
Publisher:	WILEY-V C H VERLAG GMBH
Place of Publication:	WEINHEIM
ISSN:	1521-3951
Language:	English
Faculty:	Faculty of Mathematics and Natural Sciences
Divisions:	Faculty of Mathematics and Natural Sciences > Department of Physics > Institute of Physics II
Subjects:	no entry
Uncontrolled Keywords:	Keywords Language INTERCALATION; FILMS Multiple languages Physics, Condensed Matter Multiple languages
Refereed:	Yes
URI:	http://kups.ub.uni-koeln.de/id/eprint/16333