Li, Man-Rong ORCID: 0000-0001-8424-9134, McCabe, Emma E., Stephens, Peter W., Croft, Mark, Collins, Liam, Kalinin, Sergei V., Deng, Zheng, Retuerto, Maria ORCID: 0000-0001-7564-3500, Sen Gupta, Arnab, Padmanabhan, Haricharan, Gopalan, Venkatraman, Grams, Christoph P., Hemberger, Joachim, Orlandi, Fabio ORCID: 0000-0001-6333-521X, Manuel, Pascal ORCID: 0000-0002-8845-6576, Li, Wen-Min, Jin, Chang-Qing, Walker, David and Greenblatt, Martha (2017). Magnetostriction-polarization coupling in multiferroic Mn2MnWO6. Nat. Commun., 8. LONDON: NATURE PUBLISHING GROUP. ISSN 2041-1723

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Abstract

Double corundum-related polar magnets are promising materials for multiferroic and magnetoelectric applications in spintronics. However, their design and synthesis is a challenge, and magnetoelectric coupling has only been observed in Ni3TeO6 among the known double corundum compounds to date. Here we address the high-pressure synthesis of a new polar and antiferromagnetic corundum derivative Mn2MnWO6, which adopts the Ni3TeO6-type structure with low temperature first-order field-induced metamagnetic phase transitions (T-N = 58 K) and high spontaneous polarization (similar to 63.3 mu C.cm(-2)). The magnetostrictionpolarization coupling in Mn2MnWO6 is evidenced by second harmonic generation effect, and corroborated by magnetic-field-dependent pyroresponse behavior, which together with the magnetic-field-dependent polarization and dielectric measurements, qualitatively indicate magnetoelectric coupling. Piezoresponse force microscopy imaging and spectroscopy studies on Mn2MnWO6 show switchable polarization, which motivates further exploration on magnetoelectric effect in single crystal/ thin film specimens.

Item Type: Journal Article
Creators:
CreatorsEmailORCIDORCID Put Code
Li, Man-RongUNSPECIFIEDorcid.org/0000-0001-8424-9134UNSPECIFIED
McCabe, Emma E.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Stephens, Peter W.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Croft, MarkUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Collins, LiamUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Kalinin, Sergei V.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Deng, ZhengUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Retuerto, MariaUNSPECIFIEDorcid.org/0000-0001-7564-3500UNSPECIFIED
Sen Gupta, ArnabUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Padmanabhan, HaricharanUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Gopalan, VenkatramanUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Grams, Christoph P.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Hemberger, JoachimUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Orlandi, FabioUNSPECIFIEDorcid.org/0000-0001-6333-521XUNSPECIFIED
Manuel, PascalUNSPECIFIEDorcid.org/0000-0002-8845-6576UNSPECIFIED
Li, Wen-MinUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Jin, Chang-QingUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Walker, DavidUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Greenblatt, MarthaUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
URN: urn:nbn:de:hbz:38-208022
DOI: 10.1038/s41467-017-02003-3
Journal or Publication Title: Nat. Commun.
Volume: 8
Date: 2017
Publisher: NATURE PUBLISHING GROUP
Place of Publication: LONDON
ISSN: 2041-1723
Language: English
Faculty: Faculty of Mathematics and Natural Sciences
Divisions: Faculty of Mathematics and Natural Sciences > Department of Physics > Institute of Physics II
Subjects: no entry
Uncontrolled Keywords:
KeywordsLanguage
HIGH-PRESSURE SYNTHESIS; OXYGEN OCTAHEDRAL ROTATIONS; MAGNETIC-STRUCTURE; DOMAIN-STRUCTURES; POLAR; SPIN; PEROVSKITES; BEHAVIOR; DEVICES; SYSTEMMultiple languages
Multidisciplinary SciencesMultiple languages
Refereed: Yes
URI: http://kups.ub.uni-koeln.de/id/eprint/20802

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